It's like this entire administration is made up of James Bond villains.
All right, let's break this down.
Secretary of State Rex Tillerson is Karl Stromberg.
Secretary of the Treasury Steve Mnuchin is Dr. No
Secretary of Defense Jim Mattis is Brad Whitaker
Attorney General Jeff Sessions is Dominic Greene
Secretary of the Interior Ryan Zinke is Jaws
Secretary of Agriculture Sonny Perdue is Ernst Stavro Blofeld
Secretary of Commerce Wilbur Ross is Renard
Secretary of Labor Alex Acosta is Francisco Scaramanga
HUD Secretary Dr. Ben Carson is Dr. Kananga
Secretary of Transportation Elaine Chao is Irma Bunt
Secretary of Energy Rick Perry is Ernst Stavro Blofeld (new version)
Secretary of Education Betsy DeVos is Raoul Silva
White House Chief of Staff John Kelly is Red Grant
Former White House Chief Strategist Steve Bannon is Auric Goldfinger
Former White House Deputy Assistant Seb Gorka is Hugo Drax
White House Senior Advisor Stephen Miller is Le Chiffre
Ivanka Trump and Jared Kushner are Miranda Frost and Gustav Graves (via @_datanotshown_ )
Vice President Mike Pence is Emil Largo
President Donald J. Trump is Max Zorin
All right, a few more in the wider Trumposphere.
Trump's personal lawyers Jay Sekulow and Ty Cobb are Mr. Wint and Mr. Kidd.
Trump laywer Michael Cohen is Prof. Joe Butcher
Carter Page is Zao
Former National Security Adviser General Michael Flynn as General Arkady Grigorovich Ourumov
Former Trump campaign head Paul Manafort as Kamal Khan
First Lady Melania Trump is Electra King
Counselor to the President Kellyanne Conway is Rosa Klebb

(hat tip to whoever suggested this earlier in the thread)
White House Communications Director Anthony Scaramucci is Nick Nack
White House Press Secretary Sean Spicer is General Orlov
National Security Adviser H.R. McMaster is KGB Chief A.A. Gogol
Roger Stone is Odd Job
We've come this far. Let's end this thing.
Julian Assange is Maximillian Largo
Former HHS Secretary Tom Price is Elliott Carver (played by Jonathan Pryce!)
Donald Trump Jr. and Eric Trump are Mischka and Grischka
Roger Ailes is Dr. Carl Mortner
EPA Director Scott Pruitt is Necros
And Roy Moore is Sheriff J.W. Pepper
Some final loose ends, and I'm done. I promise. Maybe.
(Fixing typos)
Sheriff David Clarke as Baron Samedi
Sheriff Joe Arpaio is Milton Krest
George Papadopolous is Carlos
Dr. Harold Bornstein is Henry Gupta
Nigel Farage is Ernst Stavro Blofeld (Diamonds Are Forever version)
Rob Goldstone is Valentin Zukov

(thanks to a comment in the replies)
Corey Lewandowski is Elvis
Katrina Pierson is Fatima Blush
Tucker Carlson is Will Truman-Lodge
Sean Hannity is General Koskov
Milo Yiannopoulos is Boris Grishenko
FCC Chairman Ajit Pai is Tee-Hee Johnson
Budget Director Mick Mulvaney is Mister Bullion
Steve Doocy and Brian Kilmeade are Bambi and Thumper
Geraldo Rivera is Angelo Palazzi
CIA Director Mike Pompeo is Alec Trevelyan
Tom Cotton is Gobinda
Trump's lawyer John Dowd is Sandor
James O'Keefe (in '70s pimp disguise) is Kananga (in Mr. Big disguise)
Paul Ryan is Mr. Stamper
Mitch McConnell is Bert Saxby
Vladimir Putin is Tov Kronsteen
Devin Nunes is Alex Dimitrios
Lindsey Graham is Pussy Galore
Chuck Grassley is Emil Locque
Press Secretary Sarah Huckabee Sanders is Mr. Kil
Secretary of Homeland Security Kirstjen Nielsen is Valenka
Nominee for Secretary of Health and Human Services Alex Azar is Sasha Davidov
Bill O'Reilly is Mr. White
Jason Chaffetz is Ed Killifer
Libertarian Party nominee Gary Johnson is Professor R.J. Dent
UN Ambassador Nikki Haley is Naomi
Jeffrey Lord is Vladimir Popov
Laura Ingraham is Jenny Flex
Governor Chris Christie is Whisper
Alex Jones is Colonel Heller
Rudy Guiliani (disguised as a blonde) is Jacques Bouvar (disguised as a blonde)
Chief Economic Adviser Gary Cohn is Ernst Stavro Blofeld (On Her Majesty's Secret Service version)
Former Chief of Staff Reince Priebus is Max Denbigh
Trump Campaign Communications Director Jason Miller is Mr. Hinx
Deputy Campaign Manager David Bossie is General Madrano
Stormy Daniels is Fiona Volpe
Florida Governor Rick Scott is Kratt
John Bolton is Gregg Beam
House Majority Leader Kevin McCarthy is Mrs. Whistler
Trump's mentor Roy Cohn is SPECTRE's Number Ten
Hugh Hewitt is Morton Slumber
Rebekah Mercer is Helga Brandt

(credit: @tottspur69)
Robert Mercer is Mr. Osato

(credit: @tottspur69)
Sheldon Adelson is Gregor Karakov
Mike Huckabee is Shady Tree
Wayne LaPierre is Adolph Gettler
White House Counsel Don McGahn is Scarpine
Fred Trump is Dr. Kaufman
Mark Halperin is Carlos Nikolic
Tiffany Trump is Bibi Dahl

(credit: @tottspur69)
Marla Maples is Jacoba Brink

(credit: @tottspur69)
Ivana Trump is Tiffany Case
Kris Kobach is Janni
White House Director of Legislative Affairs Marc Short is Trukhin
Felix Sater is Franz Sanchez
Senator Ron Johnson is Aristotle Kristatos
Rep. Matt Gaetz is Chang
Wendy Deng Murdoch is Sévérine

(credit: @Tottspur69)
Lara Trump is Verity

(credit: @Tottspur69)
Tony Perkins is Kamp
Lou Dobbs is Hans
Sarah Palin is Cigar Girl

(credit: @Tottspur69)
Rep. Jim Jordan is Patrice

(credit: @Tottspur69)
Jeanine Pirro is Gabor
Ann Coulter is Erich Kriegler
Jerry Falwell Jr. is Le Chiffre (original Orson Welles version)
Marc Kasowitz is Professor Dr. Metz
The hosts of "Fox & Friends" are the Three Blind Mice
White House Communications Strategist Mercedes Schlapp is Magda
RNC Finance Chairman Steve Wynn is Mr. Solo
RNC Chairwoman Ronna R̶o̶m̶n̶e̶y̶ McDaniel is Andrea Anders
Rep. Blake Farenthold is Aziz Fekkesh
Mike Cernovich is Krilencu
Rep. Trey Gowdy is Lazar
Scott Baio is Dario

(credit: @Tottspur69)
Sen. Marco Rubio is Mr. Jones
Deputy National Security Adviser Dina Powell is Saida

(Credit: @Tottspur69)
Sen. Ted Cruz is Count Lippe
Piers Morgan is Peter Franks
Richard Spencer is Kananga (inflated)
Rep. Steve King is Dr. Alvarez
Russian Ambassador Sergey Kislyak is Grunther

(credit: @Tottspur69)
Russian Foreign Minister Sergey Lavrov is Gumbold

(credit: @Tottspur69)
Rep. Paul Gosar, D.D.S., is Dr. Tynan, D.D.S.
Frank Gaffney is Dr. Bechmann

(credit: @Tottspur69)
Jesse Watters is François Derval
Rep. Mark Meadows is Montelongo
Newt Gingrich is Mikhail Arkov
Matt Drudge is Rodney

(credit: @Tottspur69)
Rep. Louie Gohmert is Vargas
Tomi Lahren is Stromberg's Assistant
Former Director of the Centers for Disease Control Brenda Alexander is Fiona Volpe
(I already matched Stormy Daniels to Fiona Volpe, but I'm officially changing the president's alleged porn star mistress to the more aptly-named Plenty O'Toole)
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